Dilute Magnetic Semiconductor-Ferromagnet Hybrids

S. Halm*, F. Seifert*, T. Kümmell*, Ellen Schuster*, W. Keune*, G. Bacher*, Yang-Hsiung Fan, J. Puls, and F. Henneberger

*Universität Duisburg-Essen

(DFG Projekt im Schwerpunktprogramm SPP 1133 ‚Ultraschnelle Magnetisierung’)



Nanostructured ferromagnets (FMs) provide the opportunity to manipulate spins in an underlying diluted magnetic semiconductor (DMS) heterostructure. Fringe fields from Fe/Tb FMs with a remanent out-of-plane magnetization induce a local out-of-plane magnetization in a (Zn,Cd,Mn)Se/ZnSe DMS quantum well. Due to the sp-d exchange interaction, optically generated electron-hole pairs align their spin along the DMS magnetization which is probed by both spatially resolved, polarization sensitive magneto-photoluminescence spectroscopy. Faraday rotation uncovers the alignment of the spins of the magnetic Mn ions.

S. Halm et al., Proc. E-MRS 2006 Fall Meeting, Warzawa, to appear in phys. stat. sol. (c)


The strongest vertical fringe fields can be achieved by using a planar FM with a small aperture (called an "antidot" ) To prove the spin alignment, a single 10µm x 10 µm Fe/Tb antidot structure with a 2µm x 2µm aperture is studied. The circular optical polarization degree reflecting directly the electron-hole pair (exciton) spin polarization is measured inside the aperture as a function of an externally applied magnetic field. For comparison, a DMS region without FM is investigated as a reference. The field was swept from - 5T to + 5T (open symbols) and backwards (filled symbols) and the polarization degree was measured in the relevant range from - 1T to + 1T. While there is no difference in between the up sweep and the down sweep on a DMS area without FMs, we observe a clear hysteresis in the center of the antidot with a 12% spin polarization degree at zero external field.
DMS structures on transparent ZnSe substrates allows us to perform Faraday rotation (FR) experiments on hybrid structures. FR measures the spin polarization of the magnetic Mn ions. Via the sp-d interaction, the circularly polarized exciton transitions are split energetically resulting in different phase velocity for right crcularly and left circularly polarized light. Using linearly polarized ligth, a rotation of polarization plane occurs in transmission. We studied the FR signal on a 200 µm x 200 µm array of FM antidots with 1 µm apertures and a period of 2 µm. Here, the FR signal is plotted for the antidot field at zero field (upper part) and a DMS reference area without FMs (lower part) with varying external fields at 1.5 K. Pronounced magnetic field dependent features are found at the photon energies of the heavy-hole exciton groundstate as well as the heavy-hole subband edge. The features found on the hybrid structure prove that a remanent spin polarization without external field can be realized for the magnetic Mn ions.

Previous results: H. Schömig et al., Appl. Phys. Lett. 84, 2826 (2004)